Broadband and Low-Light Photodetection in a Flexible 2d Ti3c2tx Mxene/1d-Sbsi Nanowire Heterojunction Photodetector
22 Pages Posted: 13 May 2025
Abstract
Detection of weak signals is a critical challenge for advanced applications in biomedical imaging, wearable electronics and autonomous vehicles. The efficacy of photodetectors in low light conditions is profoundly influenced by the minimization of noise current. To address this, we present a self-powered flexible photodiode (SFD) based on a Ti3C2Tx MXene/SbSI van der Waals heterojunction (vdWH). This architecture amplifies photocurrent generation while reducing noise. The vdWH interface inherent built in electric field facilitates rapid photogenerated carrier separation, achieving a responsivity of 880 mA/W together with fast response (16ms/30ms). With an ultra-low noise equivalent power (NEP) of ≈10−16 W/Hz1/2, the SFD is capable of detecting faint light signals. The SFD also enables precise heart rate monitoring via photoplethysmography (PPG) signals, offering a self-powered and non-invasive solution for early cardiovascular disease detection. This study establishes a foundation for the advancement of high-performance, MXene-based SFD architecture specifically for wearable health monitoring applications.
Keywords: 1D SbSI, 2D Ti3C2Tx MXene, heterojunction, self-powered, PPG signals
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