Broadband and Low-Light Photodetection in a Flexible 2d Ti3c2tx Mxene/1d-Sbsi Nanowire Heterojunction Photodetector

22 Pages Posted: 13 May 2025

See all articles by Muhammad Zubair Nawaz

Muhammad Zubair Nawaz

Southern University of Science and Technology

Waqas Ahmad

Shenzhen University

Asad Khaleeq

Donghua University

Waqar ul Hasan

Donghua University

Rana Zafar Abbas Manj

Donghua University

Muhammad Shahrukh Saleem

Southern University of Science and Technology

Inaam Ullah

Donghua University

Ayesha Irfan

Donghua University

Israr Masood ul Hasan

affiliation not provided to SSRN

Muhammad Yaqub

Hunan University

H. M. Noor ul Huda Khan Asghar

affiliation not provided to SSRN

Gul Naz

affiliation not provided to SSRN

Mai Li

Donghua University

Chunrui Wang

Donghua University

Yury Illarionov

Southern University of Science and Technology

Abstract

Detection of weak signals is a critical challenge for advanced applications in biomedical imaging, wearable electronics and autonomous vehicles. The efficacy of photodetectors in low light conditions is profoundly influenced by the minimization of noise current. To address this, we present a self-powered flexible photodiode (SFD) based on a Ti3C2Tx MXene/SbSI van der Waals heterojunction (vdWH). This architecture amplifies photocurrent generation while reducing noise. The vdWH interface inherent built in electric field facilitates rapid photogenerated carrier separation, achieving a responsivity of 880 mA/W together with fast response (16ms/30ms). With an ultra-low noise equivalent power (NEP) of ≈10−16 W/Hz1/2, the SFD is capable of detecting faint light signals. The SFD also enables precise heart rate monitoring via photoplethysmography (PPG) signals, offering a self-powered and non-invasive solution for early cardiovascular disease detection. This study establishes a foundation for the advancement of high-performance, MXene-based SFD architecture specifically for wearable health monitoring applications.

Keywords: 1D SbSI, 2D Ti3C2Tx MXene, heterojunction, self-powered, PPG signals

Suggested Citation

Nawaz, Muhammad Zubair and Ahmad, Waqas and Khaleeq, Asad and Hasan, Waqar ul and Abbas Manj, Rana Zafar and Saleem, Muhammad Shahrukh and Ullah, Inaam and Irfan, Ayesha and Hasan, Israr Masood ul and Yaqub, Muhammad and Khan Asghar, H. M. Noor ul Huda and Naz, Gul and Li, Mai and Wang, Chunrui and Illarionov, Yury, Broadband and Low-Light Photodetection in a Flexible 2d Ti3c2tx Mxene/1d-Sbsi Nanowire Heterojunction Photodetector. Available at SSRN: https://ssrn.com/abstract=5246727 or http://dx.doi.org/10.2139/ssrn.5246727

Muhammad Zubair Nawaz (Contact Author)

Southern University of Science and Technology ( email )

No 1088, xueyuan Rd.
Xili, Nanshan District
Shenzhen, 518055
China

Waqas Ahmad

Shenzhen University ( email )

3688 Nanhai Road, Nanshan District
Shenzhen, 518060
China

Asad Khaleeq

Donghua University ( email )

Shanghai 200051
China

Waqar ul Hasan

Donghua University ( email )

Shanghai 200051
China

Rana Zafar Abbas Manj

Donghua University ( email )

Shanghai 200051
China

Muhammad Shahrukh Saleem

Southern University of Science and Technology ( email )

No 1088, xueyuan Rd.
Xili, Nanshan District
Shenzhen, 518055
China

Inaam Ullah

Donghua University ( email )

Ayesha Irfan

Donghua University ( email )

Israr Masood ul Hasan

affiliation not provided to SSRN ( email )

Muhammad Yaqub

Hunan University ( email )

2 Lushan South Rd
Changsha, CA 410082
China

H. M. Noor ul Huda Khan Asghar

affiliation not provided to SSRN ( email )

Gul Naz

affiliation not provided to SSRN ( email )

Mai Li

Donghua University ( email )

Chunrui Wang

Donghua University ( email )

Yury Illarionov

Southern University of Science and Technology ( email )

No 1088, xueyuan Rd.
Xili, Nanshan District
Shenzhen, 518055
China

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